1.1
This test method covers procedures for measuring reaction rates by assaying a fission product (F.P.) from the fission reaction
238
U(n,f)F.P.
1.2
The reaction is useful for measuring neutrons with energies from approximately 1.5 to 7 MeV and for irradiation times up to 30 to 40 years, provided that the analysis methods described in Practice
E261
are followed.
1.3
Equivalent fission neutron fluence rates as defined in Practice
E261
can be determined.
1.4
Detailed procedures for other fast-neutron detectors are referenced in Practice
E261
.
1.5
The values stated in SI units are to be regarded as standard. No other units of measurement are included in this standard.
1.6
This standard does not purport to address all of the safety concerns, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety, health, and environmental practices and determine the applicability of regulatory limitations prior to use.
1.7
This international standard was developed in accordance with internationally recognized principles on standardization established in the Decision on Principles for the Development of International Standards, Guides and Recommendations issued by the World Trade Organization Technical Barriers to Trade (TBT) Committee.
====== Significance And Use ======
5.1
Refer to Practice
E261
for a general discussion of the determination of fast-neutron fluence rate with fission detectors.
5.2
238
U is available as metal foil, wire, or oxide powder (see Guide
E844
). It is usually encapsulated in a suitable container to prevent loss of, and contamination by, the
238
U and its fission products.
5.3
One or more fission products can be assayed. Pertinent data for relevant fission products are given in
Table 1
and
Table 2
.
(A)
The lightface numbers in parentheses are the magnitude of plus or minus uncertainties in the last digit(s) listed.
(B)
With
137m
Ba (2.552 min) in equilibrium.
(C)
The recommended half-life and gamma emission probabilities have been taken from the Reference
(
3
)
data that was recommended at the time that the recommended fission yields were set.
(D)
Probability of daughter
140
La decay.
(E)
This is the activity ratio of
140
La/
140
Ba after reached transient equilibrium (t
≥
19 days).
(A)
The JEFF-3.1/3.1.1 radioactive decay data and fission yields sub-libraries, JEFF Report 20, OECD 2009, Nuclear Energy Agency
(
5
)
.
(B)
All yield data given as a %; RC represents a cumulative yield; RI represents an independent yield.
5.3.1
137
Cs-
137m
Ba is chosen frequently for long irradiations. Radioactive products
134
Cs and
136
Cs may be present, which can interfere with the counting of the 0.662 MeV
137
Cs-
137m
Ba gamma rays (see Test Method
E320
).
5.3.2
140
Ba-
140
La is chosen frequently for short irradiations (see Test Method
E393
).
5.3.3
95
Zr can be counted directly, following chemical separation, or with its daughter
95
Nb using a high-resolution gamma detector system.
5.3.4
144
Ce is a high-yield fission product applicable to 2- to 3-year irradiations.
5.4
It is necessary to surround the
238
U monitor with a thermal neutron absorber to minimize fission product production from a quantity of
235
U in the
238
U target and from
239
Pu from (n,γ) reactions in the
238
U material. Assay of the
239
Pu concentration when a significant contribution is expected.
5.4.1
Fission product production in a light-water reactor by neutron activation product
239
Pu has been calculated to be insignificant (<2 %), compared to that from
238
U(n,f), for an irradiation period of 12 years at a fast-neutron (
E
> 1 MeV) fluence rate of 1 × 10
11
cm
−2
· s
−1
provided the
238
U is shielded from thermal neutrons (see Fig. 2 of Guide
E844
).
5.4.2
Fission product production from photonuclear reactions, that is, (γ,f) reactions, while negligible near-power and research-reactor cores, can be large for deep-water penetrations
(
6
)
.
4
5.5
Good agreement between neutron fluence measured by
238
U fission and the
54
Fe(n,p)
54
Mn reaction has been demonstrated
(
7
)
. The reaction
238
U(n,f) F.P. is useful since it is responsive to a broader range of neutron energies than most threshold detectors.
5.6
The
238
U fission neutron spectrum-averaged cross section in several benchmark neutron fields is given in Table 3 of Practice
E261
. Sources for the latest recommended cross sections are given in Guide
E1018
. In the case of the
238
U(n,f)F.P. reaction, the recommended cross section source is the ENDF/B-VI release 8 cross section (MAT = 9237)
(
8
)
.
Fig. 1
shows a plot of the recommended cross section versus neutron energy for the fast-neutron reaction
238
U(n,f)F.P.
FIG. 1
ENDF/B-VI Cross Section Versus Energy for the
238
U(n,f)F.P. Reaction
Note 1:
The data is taken from the Evaluated Nuclear Data File, ENDF/B-VI, rather than the later ENDF/B-VII. This is in accordance with Guide
E1018
, Section 6.1, since the later ENDF/B-VII data files do not include covariance information. Some covariance information exists for
238
U in the standard sublibrary, but this is only for energies greater than 1 MeV. For more details, see Section H of Ref
9
.